22-Alkyl-20-epi-1alpha,25-dihydroxyvitamin D3 compounds of superagonistic activity: syntheses, biological activities and interaction with the receptor

J Med Chem. 2007 Mar 8;50(5):932-9. doi: 10.1021/jm060889f. Epub 2007 Feb 14.

Abstract

We previously reported that 22R-methyl-20-epi-1,25-(OH)2D3 (3) possesses strong binding affinity for the vitamin D receptor (VDR) and shows superagonistic biological activities. To examine the effect of the length of an alkyl substituent at C(22) and to extend our compound library, we successfully synthesized 22R-ethyl-20-epi-1,25-(OH)2D3 (4) and 22R-butyl-20-epi-1,25-(OH)2D3 (5). Surprisingly, 22-ethyl analogue 4 showed stronger VDR binding affinity and transactivation potency than the superagonist of methyl analogue 3, but its calcemic activity in vivo was weaker than that of both the methyl analogue 3 and the natural hormone (1), while 22-butyl analogue 5 showed activities comparable to those of the hormone (1). A study of the docking of these new analogues to the VDR-LBD and alanine scanning mutational analysis demonstrated that 22-methyl and 22-ethyl substituents enhance the favorable hydrophobic interactions with residues lining the ligand binding pocket of the VDR, and that 22-butyl analogue 5 binds to the VDR by an induced fit mechanism.

MeSH terms

  • Animals
  • Binding Sites
  • Biological Transport
  • Bone and Bones / metabolism
  • COS Cells
  • Calcitriol / analogs & derivatives*
  • Calcitriol / chemical synthesis
  • Calcitriol / chemistry
  • Calcitriol / pharmacology
  • Calcium / metabolism
  • Cattle
  • Cell Differentiation / drug effects
  • Chlorocebus aethiops
  • HL-60 Cells
  • Humans
  • In Vitro Techniques
  • Intestinal Mucosa / metabolism
  • Ligands
  • Models, Molecular
  • Mutation
  • Radioligand Assay
  • Rats
  • Receptors, Calcitriol / antagonists & inhibitors*
  • Receptors, Calcitriol / genetics
  • Stereoisomerism
  • Structure-Activity Relationship
  • Transcriptional Activation / drug effects

Substances

  • 22-butyl-1,25-dihydroxyvitamin D3
  • 22-ethyl-1,25-dihydroxyvitamin D3
  • Ligands
  • Receptors, Calcitriol
  • Calcitriol
  • Calcium